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Amino-Supported Palladium Catalyst for Chemo- and Stereoselective Domino Reactions
Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Anhui, Peoples R China..
Stockholm Univ, Dept Organ Chem, Arrhenius Lab, SE-10691 Stockholm, Sweden..
Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Anhui, Peoples R China..
Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Anhui, Peoples R China..
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2021 (English)In: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 60, no 2, p. 670-674Article in journal (Refereed) Published
Abstract [en]

A solid amino-supported palladium catalyst is used in an oxidative domino reaction for the diastereoselective construction of alkyne-substituted cyclopentenol compounds. This heterogeneous catalyst exhibits high efficiency and excellent chemoselectivity, as well as good recyclability. The chemoselectivity of the domino reactions was readily controlled by switching the solvent and catalyst. Asymmetric syntheses and an oxidative carbocyclization-borylation reaction have also been developed based on the heterogeneous palladium catalyst.
Place, publisher, year, edition, pages
2021. Vol. 60, no 2, p. 670-674
Keywords [en]
amines, cyclizations, heterogeneous catalysis, palladium, supported catalysts
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:miun:diva-40616DOI: 10.1002/anie.202011708ISI: 000587743800001PubMedID: 32969105Scopus ID: 2-s2.0-85096704318OAI: oai:DiVA.org:miun-40616DiVA, id: diva2:1504225
Available from: 2020-11-27 Created: 2020-11-27 Last updated: 2025-09-25

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Bäckvall, Jan-Erling

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