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  • 1.
    Hedenstedt, Kristoffer
    et al.
    Göteborgs Universitet; AkzoNobel.
    Bäckström, Joakim
    Mittuniversitetet, Fakulteten för naturvetenskap, teknik och medier, Avdelningen för naturvetenskap. Göteborgs Universitet.
    Ahlberg, Elisabet
    Göteborgs Universitet.
    In-Situ Raman Spectroscopy of α- and γ-FeOOH during Cathodic Load2017Inngår i: Journal of the Electrochemical Society, ISSN 0013-4651, E-ISSN 1945-7111, Vol. 164, nr 9, s. H621-H627Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Water reduction on corroded iron surfaces is technologically and fundamentally important. Here, the technological interest originatesfrom the chlorate process where water reduction is the main cathodic process. Fundamentally, water reduction on oxide surfaces raisesquestions on the stability of the oxide and the nature of electrocatalytic surface sites. Two iron oxyhydroxides,α-andγ-FeOOH,were electrodeposited on titanium substrate and their reduction processes were followed in detail with in-situ Raman spectroscopy,using low incident laser power to avoid sample damaging. Polarization to negative potentials show two reduction peaks forγ-FeOOHand one peak forα-FeOOH prior to hydrogen evolution. The characteristic Raman peaks gradually disappear as the potential ismade more negative but no new peaks can be observed.δ-FeOOH was detected as an intermediate phase upon oxidation of thereduced surface layer. This indicates that Fe(OH)2is formed during cathodic polarization and initially re-oxidized to the isostructuralδ-FeOOH. Characteristic Raman signals of the original phases appear upon further oxidation in air.

  • 2. Nozière, Barbara
    et al.
    Dziedzic, Pawel
    Córdova, Armando
    Mittuniversitetet, Fakulteten för naturvetenskap, teknik och medier, Institutionen för naturvetenskap, teknik och matematik.
    Common Inorganic Ions Catalyze Chemical Reactions of Organic Compounds in Atmospheric Aerosols2010Inngår i: Physical Chemistry, Chemical Physics - PCCP, ISSN 1463-9076, E-ISSN 1463-9084, Vol. 12, s. 3864-Artikkel i tidsskrift (Fagfellevurdert)
  • 3.
    van Hees, P A W
    et al.
    Mittuniversitetet, Fakulteten för naturvetenskap, teknik och medier, Institutionen för naturvetenskap.
    Godbold, D L
    Jentschke, G
    Jones, D L
    Impact of ectomycorrhizas on the concentration and biodegradation of simple organic acids in a forest soil2003Inngår i: European Journal of Soil Science, ISSN 1351-0754, E-ISSN 1365-2389, Vol. 54, nr 4, s. 697-706Artikkel i tidsskrift (Fagfellevurdert)
    Abstract [en]

    Simple organic acids seem to be important in many soil processes including nutrient uptake in the rhizosphere and long-term pedogenic processes such as podzolization. The factors regulating the concentrations of these acids in soil, however, remain poorly understood. We have investigated one set of factors, namely the impact of ectomycorrhizal (Paxillus involutus) and non-mycorrhizal Picea abies seedlings and humic acid on the concentration and dynamics of organic acids in soil solution. We did so over 10 months in laboratory columns containing soil from the E horizon of a sandy forest soil. Several organic acids were identified in the solution extracted from the root zone including oxalic, citric, malonic, succinic, acetic, formic and lactic acids at concentrations ranging from <0.1 to 2.3 muM. Both plants and ectomycorrhizas had significant effects on the concentration of organic acids in soil solution. In contrast, omitting P from the irrigation water appeared to have little effect on the concentrations. The microbial mineralization kinetics of oxalate conformed well to a single Michaelis-Menten equation. Further, the soil with the mycorrhizas had a significantly faster mineralization of oxalic acid over a wide concentration range than did the soil without ectomycorrhizas and without plants. We conclude that the oxalate flux through the soil with both trees and mycorrhizas is much faster than is evident from measurements of solution concentration at steady state. Humic acid had little effect on the concentrations of organic acids or dynamics in the soil solution. Oxalic acid concentrations in the soil solution were correlated with hyphal length, rate of microbial mineralization, soil respiration, and shoot to root weight ratio. We conclude that both mycorrhizas and plants have a large impact on organic acid cycling in forest soils.

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