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Enantioselective Heterogeneous Synergistic Catalysis for Asymmetric Cascade Transformations
Department of Organic Chemistry, Arrhenius Laboratory, Stockholm University, 106 91 Stockholm, Sweden.
Department of Organic Chemistry, Arrhenius Laboratory, Stockholm University, 106 91 Stockholm, Sweden.
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences.ORCID iD: 0000-0002-5108-6487
Department of Organic Chemistry, Arrhenius Laboratory, Stockholm University, 106 91 Stockholm, Sweden.
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2014 (English)In: Advanced Synthesis and Catalysis, ISSN 1615-4150, E-ISSN 1615-4169, Vol. 356, no 11-12, p. 2485-2492Article in journal (Refereed) Published
Abstract [en]

A modular design for a novel heterogeneous synergistic catalytic system, which simultaneously activates the electrophile and nucleophile by the combined activation modes of a separate metal and non-metal catalyst, for asymmetric cascade transformations on a solid surface is disclosed. This modular catalysis strategy generates carbocycles (up to 97.5: 2.5 er) as well as spirocyclic oxindoles (97.5: 2.5 to > 99: 0.5 er), containing all-carbon quaternary centers, in a highly enantioselective fashion via a one-pot dynamic relay process.

Place, publisher, year, edition, pages
2014. Vol. 356, no 11-12, p. 2485-2492
Keywords [en]
all-carbon quaternary stereocenters, carbocycles, co-catalysis, dynamic transformations, heterogeneous synergistic catalysis
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:miun:diva-23017DOI: 10.1002/adsc.201400291ISI: 000340567100014Scopus ID: 2-s2.0-84906246251OAI: oai:DiVA.org:miun-23017DiVA, id: diva2:748157
Available from: 2014-09-18 Created: 2014-09-18 Last updated: 2017-12-05Bibliographically approved

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Afewerki, SamsonCordova, Armando

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