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Palladium/Chiral Amine Co-catalyzed Enantioselective beta-Arylation of alpha,beta-Unsaturated Aldehydes
Mid Sweden University, Faculty of Science, Technology and Media, Department of Chemical Engineering.
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences. (Armando Córdova)
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences. (Armando Córdova)ORCID iD: 0000-0002-5108-6487
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences. (Armando Córdova)
2013 (English)In: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 52, no 3, p. 878-882Article in journal (Refereed) Published
Abstract [en]

Palladium and a simple chiral amine are used as co-catalysts for the enantioselective conjugate addition of aryl boronic acids to α,β-unsaturated aldehydes (see scheme). The synthetic utility of this co-catalyzed reaction was demonstrated in the short total syntheses of (R)-(-)-curcumene and 4-aryl-2-ones. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Place, publisher, year, edition, pages
2013. Vol. 52, no 3, p. 878-882
Keywords [en]
aldehydes; asymmetric catalysis; boronic acids; co-catalysts; total synthesis
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:miun:diva-18083DOI: 10.1002/ange.201208634ISI: 000313688100012Scopus ID: 2-s2.0-84872316330OAI: oai:DiVA.org:miun-18083DiVA, id: diva2:580136
Note

Article first published online: 23 NOV 2012

Available from: 2012-12-20 Created: 2012-12-20 Last updated: 2017-12-06Bibliographically approved

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Ibrahem, IsmailMa, GuangningAfewerki, SamsonCórdova, Armando

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