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Assigning x-ray absorption spectra by means of soft-x-ray emission spectroscopy
Mid Sweden University.
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1998 (English)In: Physical Review A. Atomic, Molecular, and Optical Physics, ISSN 1050-2947, Vol. 57, no 2, 864-872 p.Article in journal (Refereed) Published
Abstract [en]

The possibility to symmetry assign x-ray absorption spectra using x-ray emission spectroscopy is demonstrated. The oxygen K spectra of CO2 are used to illustrate the possibility to assign core excitations through excitation-energy and angular dependence of resonantly excited x-ray emission spectra. The Rydberg-associated structures just below the ionization threshold in the O K x-ray absorption spectrum are assigned to be mainly due to excitations to orbitals of sigma(g) character. The results, which contradict some previous literature assignments, are supported by quantum-chemical calculations.

Place, publisher, year, edition, pages
1998. Vol. 57, no 2, 864-872 p.
Keyword [en]
HIGH-RESOLUTION, SYMMETRY-BREAKING, MOLECULAR-OXYGEN, STATIC EXCHANGE, CO2, POLARIZATION, FLUORESCENCE, ANISOTROPY, RESONANCES
National Category
Natural Sciences
Identifiers
URN: urn:nbn:se:miun:diva-2085Local ID: 1093OAI: oai:DiVA.org:miun-2085DiVA: diva2:27117
Available from: 2008-09-30 Created: 2008-09-30 Last updated: 2011-01-10Bibliographically approved

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