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Highly Diastereo- and Enantioselective Cascade Synthesis of Bicyclic Lactams in One-Pot
Stockholm University, Stockholm.
Stockholm University, Stockholm.
Stockholm University, Stockholm.
Stockholm University, Stockholm.
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2018 (English)In: European Journal of Organic Chemistry, ISSN 1434-193X, E-ISSN 1099-0690, Vol. 2018, no 9, p. 1158-1164Article in journal (Refereed) Published
Abstract [en]

A versatile and highly stereoselective synthetic route to functionalized bi- and tricyclic lactams (up to > 20:1 dr and 99 % ee) in one pot from simple starting materials (allylic alcohols, enals, diamines and amino alcohols) using cascade transformations promoted by chiral amine/Brønsted or metal/chiral amine/Brønsted relay catalysis is disclosed. Here molecular oxygen is employed as the terminal oxidant for the latter relay catalysis approach. 

Place, publisher, year, edition, pages
2018. Vol. 2018, no 9, p. 1158-1164
Keywords [en]
Aminal, Asymmetric catalysis, Bicyclic lactams, Hemiaminal ether, Relay catalysis
National Category
Organic Chemistry
Identifiers
URN: urn:nbn:se:miun:diva-33305DOI: 10.1002/ejoc.201701789ISI: 000426771400009Scopus ID: 2-s2.0-85043233373OAI: oai:DiVA.org:miun-33305DiVA, id: diva2:1191607
Available from: 2018-03-19 Created: 2018-03-19 Last updated: 2018-04-03Bibliographically approved

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Córdova, Armando

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