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Role of screening and angular distributions in resonant x-ray emission of CO
Mittuniversitetet.
Vise andre og tillknytning
1997 (engelsk)Inngår i: Physical Review A. Atomic, Molecular, and Optical Physics, ISSN 1050-2947, Vol. 55, nr 1, s. 134-145Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Resonantly excited carbon and oxygen x-ray-emission spectra of gaseous carbon monoxide are presented. Emission spectra obtained with selective excitation to the pi* valence orbital and to various Rydberg levels are compared to satellite-free nonresonant spectra. Screening effects caused by the excited electron, creating energy shifts and intensity variations in the resonant spectra compared to the nonresonant spectra, are observed, as well as an angular dependence of the resonantly excited spectra. The experimental spectra are compared to simulated spectra where the vibronic part is computed by means of a lifetime-vibrational interference formalism. The electronic intensities are analyzed by a separate-state, self-consistent-held method and a formalism for resonant inelastic x-ray scattering, focusing On screening and angular dependence.

sted, utgiver, år, opplag, sider
1997. Vol. 55, nr 1, s. 134-145
Emneord [en]
K-SHELL EXCITATION, HIGH-RESOLUTION, SYNCHROTRON-RADIATION, VIBRATIONAL STRUCTURE, WAVE-FUNCTIONS, SPECTRA, FLUORESCENCE, MOLECULES, SYMMETRY, CARBON
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Identifikatorer
URN: urn:nbn:se:miun:diva-1678Lokal ID: 1096OAI: oai:DiVA.org:miun-1678DiVA, id: diva2:26710
Tilgjengelig fra: 2008-09-30 Laget: 2008-09-30 Sist oppdatert: 2011-01-10bibliografisk kontrollert

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