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Catalytic Enantioselective Synthesis of Bicyclic Lactam N,S-Acetals in One Pot by Cascade Transformations
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences.
Mid Sweden University, Faculty of Science, Technology and Media, Department of Natural Sciences.
Stockholm University, Stockholm.
Stockholm University, Stockholm.
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2019 (English)In: European Journal of Organic Chemistry, ISSN 1434-193X, E-ISSN 1099-0690, Vol. 2019, no 29, p. 4649-4657Article in journal (Refereed) Published
Abstract [en]

A versatile strategy for the enantioselective synthesis of bicyclic lactam N,S-acetals by one-pot cascade transformations is disclosed. The transformation of readily available substrates is promoted by chiral amines and creates bicyclic or tricyclic lactam N,S-acetals with high chemo- and stereoselectivity (up to > 99.5:0.5 dr and > 99 % ee) in one-pot operations.

Place, publisher, year, edition, pages
2019. Vol. 2019, no 29, p. 4649-4657
Keywords [en]
Acetals, Asymmetric catalysis, Lactams, Multicomponent reactions, Synthetic methods
Identifiers
URN: urn:nbn:se:miun:diva-36896DOI: 10.1002/ejoc.201900923ISI: 000479612000001Scopus ID: 2-s2.0-85070108110OAI: oai:DiVA.org:miun-36896DiVA, id: diva2:1344055
Available from: 2019-08-20 Created: 2019-08-20 Last updated: 2019-09-02Bibliographically approved

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Zhang, KeihangDeiana, LucaCórdova, Armando

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