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Zhang, R., Hummelgård, M., Örtegren, J., Olsen, M., Andersson, H. & Olin, H. (2019). Interaction of the human body with triboelectric nanogenerators. Nano Energy, 57, 279-292
Open this publication in new window or tab >>Interaction of the human body with triboelectric nanogenerators
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2019 (English)In: Nano Energy, ISSN 2211-2855, E-ISSN 2211-3282, Vol. 57, p. 279-292Article in journal (Refereed) Published
Abstract [en]

The use of triboelectric nanogenerators (TENGs) is a new technique for energy harvesting at both small and large scales. Almost all types of mechanical energy can be harvested with TENGs by using four modes of operation that cover almost all mechanical motions. The interactions of the human body with TENGs range from energy harvesting, motion sensing, and biomedical applications to human-computer communications. Different types of TENGs have been developed to directly or indirectly involve the human body. This review will summarize the recent advances in the interaction of the human body with TENGs.

Keywords
Energy harvesting, Healthcare, Human body, Human-robot interactions, Sensors, Triboelectric nanogenerators
National Category
Other Physics Topics
Identifiers
urn:nbn:se:miun:diva-35386 (URN)10.1016/j.nanoen.2018.12.059 (DOI)000458419000028 ()2-s2.0-85059038089 (Scopus ID)
Available from: 2019-01-06 Created: 2019-01-06 Last updated: 2019-03-18Bibliographically approved
Rastabi, S. A., Mamoory, R. S., Dabir, F., Blomquist, N., Phadatare, M. R. & Olin, H. (2019). Synthesis of NiMoO4/3D-rGO Nanocomposite in Alkaline Environments for Supercapacitor Electrodes. Crystals, 9(1), Article ID 31.
Open this publication in new window or tab >>Synthesis of NiMoO4/3D-rGO Nanocomposite in Alkaline Environments for Supercapacitor Electrodes
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2019 (English)In: Crystals, ISSN 2073-4352, Vol. 9, no 1, article id 31Article in journal (Refereed) Published
Abstract [en]

Although Graphene oxide (GO)-based materials is known as a favorable candidate for supercapacitors, its conductivity needs to be increased. Therefore, this study aimed to investigate the performance of GO-based supercapicitor with new methods. In this work, an ammonia solution has been used to remove the oxygen functional groups of GO. In addition, a facile precipitation method was performed to synthesis a NiMoO4/3D-rGO electrode with purpose of using synergistic effects of rGO conductivity properties as well as NiMoO4 pseudocapacitive behavior. The phase structure, chemical bands and morphology of the synthesized powders were investigated by X-ray diffraction (XRD), Raman spectroscopy, and field emission secondary electron microscopy (FE-SEM). The electrochemical results showed that the NiMoO4/3D-rGO(II) electrode, where ammonia has been used during the synthesis, has a capacitive performance of 932 Fg(-1). This is higher capacitance than NiMoO4/3D-rGO(I) without using ammonia. Furthermore, the NiMoO4/3D-rGO(II) electrode exhibited a power density of up to 17.5 kW kg(-1) and an energy density of 32.36 Wh kg(-1). These results showed that ammonia addition has increased the conductivity of rGO sheets, and thus it can be suggested as a new technique to improve the capacitance.

Keywords
renewable energy systems, pseudocapacitive behavior, electrochemical results, ammonia, oxygen groups
National Category
Chemical Engineering
Identifiers
urn:nbn:se:miun:diva-35806 (URN)10.3390/cryst9010031 (DOI)000458578100031 ()
Available from: 2019-03-19 Created: 2019-03-19 Last updated: 2019-03-19Bibliographically approved
Andres, B., Dahlström, C., Blomquist, N., Norgren, M. & Olin, H. (2018). Cellulose binders for electric double-layer capacitor electrodes: The influence of cellulose quality on electrical properties. Materials & design, 141, 342-349
Open this publication in new window or tab >>Cellulose binders for electric double-layer capacitor electrodes: The influence of cellulose quality on electrical properties
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2018 (English)In: Materials & design, ISSN 0264-1275, E-ISSN 1873-4197, Vol. 141, p. 342-349Article in journal (Refereed) Published
Abstract [en]

Cellulose derivatives are widely used as binders and dispersing agents in different applications. Binders composed of cellulose are an environmentally friendly alternative to oil-based polymer binding agents. Previously, we reported the use of cellulose nanofibers (CNFs) as binders in electrodes for electric double-layer capacitors (EDLCs). In addition to good mechanical stability, we demonstrated that CNFs enhanced the electrical performance of the electrodes. However, cellulose fibers can cover a broad range of length scales, and the quality requirements from an electrode perspective have not been thoroughly investigated. To evaluate the influence of fiber quality on electrode properties, we tested seven samples with different fiber dimensions that are based on the same kraft pulp. To capture the length scale from fibers to nanofibrils, we evaluated the performance of the untreated kraft pulp, refined fibers, microfibrillated cellulose (MFC) and CNFs. Electrodes with kraft pulp or refined fibers showed the lowest electrical resistivity. The specific capacitances of all EDLCs were surprisingly similar, but slightly lower for the EDLC with CNFs. The same electrode sample with CNFs also showed a slightly higher equivalent series resistance (ESR), compared to those of the other EDLCs. Graphite dispersions with MFC showed the best dispersion stability. 

Keywords
Cellulose, Electric double-layer capacitor, Graphite, Nanocellulose, Nanocomposite, Supercapacitor
National Category
Chemical Engineering
Identifiers
urn:nbn:se:miun:diva-32766 (URN)10.1016/j.matdes.2017.12.041 (DOI)000424945300031 ()2-s2.0-85040002856 (Scopus ID)
Available from: 2018-01-30 Created: 2018-01-30 Last updated: 2018-07-19Bibliographically approved
Zhang, R., Carlsson, F., Edman, M., Hummelgård, M., Jonsson, B.-G., Bylund, D. & Olin, H. (2018). Escherichia coli Bacteria Develop Adaptive Resistance to Antibacterial ZnO Nanoparticles. Advanced Biosystem, 2(5), Article ID 1800019.
Open this publication in new window or tab >>Escherichia coli Bacteria Develop Adaptive Resistance to Antibacterial ZnO Nanoparticles
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2018 (English)In: Advanced Biosystem, ISSN 2366-7478, Vol. 2, no 5, article id 1800019Article in journal (Refereed) Published
Abstract [en]

Antibacterial agents based on nanoparticles (NPs) have many important applications, e.g., for the textile industry, surface disinfection, wound dressing, water treatment, and food preservation. Because of their prevalent use it is important to understand whether bacteria could develop resistance to such antibacterial NPs similarly to the resistance that bacteria are known to develop to antibiotics. Here, it is reported that Escherichia coli(E. coli) develops adaptive resistance to antibacterial ZnO NPs after several days' exposure to the NPs. But, in contrast to antibiotics‐resistance, the observed resistance to ZnO NPs is not stable—after several days without exposure to the NPs, the bacteria regain their sensitivity to the NPs' antibacterial properties. Based on the analyses it is suggested that the observed resistance is caused by changes in the shape of the bacteria and the expressions of membrane proteins. The findings provide insights into the response of bacteria to antibacterial NPs, which is important to elucidate for designing and evaluating the risk of applications based on antibacterial NPs.

Place, publisher, year, edition, pages
John Wiley & Sons, 2018
National Category
Nano Technology
Identifiers
urn:nbn:se:miun:diva-34436 (URN)10.1002/adbi.201800019 (DOI)000446970000008 ()
Available from: 2018-09-18 Created: 2018-09-18 Last updated: 2018-11-19Bibliographically approved
Zhang, R., Örtegren, J., Hummelgård, M., Olsen, M., Andersson, H. & Olin, H. (2018). Harvesting triboelectricity from the human body using non-electrode triboelectric nanogenerators. Nano Energy, 45, 298-303
Open this publication in new window or tab >>Harvesting triboelectricity from the human body using non-electrode triboelectric nanogenerators
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2018 (English)In: Nano Energy, ISSN 2211-2855, E-ISSN 2211-3282, Vol. 45, p. 298-303Article in journal (Refereed) Published
Abstract [en]

Triboelectrification has been known and discussed since antiquity. Triboelectrification occurs in the human body due to friction between human skin and other materials such as clothing. However, charges on the body have not been harvested to power small electronics. Here, we report for the first time that the electricity generated on the human body due to triboelectrification can be measured and harvested using human body-based non-electrode triboelectric nanogenerators (H-TENGs). The H-TENGs can have an output of up to 3.3 W/m(2) and can spontaneously harvest energy from several people. The functions of the human body in the H-TENGs are analyzed and experimentally proven to be those of a triboelectric material, conductor and capacitor. Our results demonstrate that the triboelectricity generated on a human body can be harvested using H-TENGs and provide scientific insights into body functions that will promote further studies of TENGs.

Keywords
Human body, Non-electrode TENG, Mechanisms, Charges
National Category
Medical Biotechnology
Identifiers
urn:nbn:se:miun:diva-33301 (URN)10.1016/j.nanoen.2017.12.053 (DOI)000425396400033 ()2-s2.0-85043782783 (Scopus ID)
Available from: 2018-03-19 Created: 2018-03-19 Last updated: 2018-03-28Bibliographically approved
Zhang, R., Engholm, M., Hummelgård, M., Andersson, H., Örtegren, J. & Olin, H. (2018). High-performance transparent and flexible electrodes made by flash-light sintering of gold nanoparticles. ACS Applied Energy Materials, 1(12), 7191-7198
Open this publication in new window or tab >>High-performance transparent and flexible electrodes made by flash-light sintering of gold nanoparticles
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2018 (English)In: ACS Applied Energy Materials, E-ISSN 2574-0962, Vol. 1, no 12, p. 7191-7198Article in journal (Refereed) Published
Abstract [en]

Metallic nanowire-based transparent electrodes (TEs) are potential alternatives to indium tin oxide (ITO). To achieve a high performance [sheet resistance (Rs) < 100 Ω/sq, transmittance (T%) > 90%], the nanowires must have a high length-to-diameter (L/D) ratio to minimize the number of wire-to-wire junctions. Attempts to produce TEs with gold nanowires have been made, and the results reveal difficulties in achieving the requirements. A successful strategy involves creating templated gold nanonetworks through multiple procedures. Here, we present a simple and efficient method that uses flash-light sintering of a gold nanonetwork film into gold TEs (Rs: 82.9 Ω/sq, T %: 91.79%) on a thin polycarbonate film (25 μm). The produced gold TEs have excellent mechanical, electrical, optical, and chemical stabilities. Mechanisms of the formation of gold nanonetworks and the effect of flash-light have been analyzed. Our findings provide a scalable process for producing transparent and flexible gold electrodes with a total processing time of less than 8 min without the use of heating, vacuum processing, and organic chemicals and without any material loss. This is possible because all the gold nanoparticles have been aggregated and filtrated on the filter membranes. The area density of gold is 0.094 g/m2 leading low material costs, which is very competitive with the price of commercial TEs.

Keywords
transparent electrode, flexible electrode, gold nanoparticles, flash-light sintering, high performance
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:miun:diva-35380 (URN)10.1021/acsaem.8b01649 (DOI)000458706800063 ()
Available from: 2019-01-03 Created: 2019-01-03 Last updated: 2019-03-15Bibliographically approved
Zhang, R., Hummelgård, M., Örtegren, J., Olsen, M., Andersson, H., Yang, Y. & Olin, H. (2018). Human body constituted triboelectric nanogenerators as energy harvesters, code transmitters and motion sensors. ACS Applied Energy Materials, 1(6), 2955-2960
Open this publication in new window or tab >>Human body constituted triboelectric nanogenerators as energy harvesters, code transmitters and motion sensors
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2018 (English)In: ACS Applied Energy Materials, ISSN 2574-0962, Vol. 1, no 6, p. 2955-2960Article in journal (Refereed) Published
Abstract [en]

Human skin is a dielectric material that can be used as a triboelectric material for harvesting energy from body motions. The output power of such a human skin-based triboelectric nanogenerator (TENG) is relatively low. Here, we assembled high-output human body constituted TENGs (H-TENGs) by taking advantage of the unique electrical properties of the human body, such as high skin impedance, low tissue resistance, body capacitance, and conductivity. The output of a H-TENG can reach 30 W/m2, which is enough to drive small electronic devices, such as a timer or a calculator. The unique feature of the H-TENG is that it can perform the four fundamental modes of TENGs, which has not been reported elsewhere. Such a feature allows the H-TENG to act as a code transmitter to send light and electrical signals, such as Morse code. H-TENGs also benefit the development of high-performance, self-powered body motion sensors. Our findings suggest new strategies for harvesting energy from human body motions, as well as new types of motion sensors and signal senders.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2018
Keywords
code transmitters; energy harvesting; human body; motion sensors; triboelectric nanogenerators
National Category
Other Physics Topics
Identifiers
urn:nbn:se:miun:diva-34433 (URN)10.1021/acsaem.8b00667 (DOI)000458705800070 ()
Available from: 2018-09-18 Created: 2018-09-18 Last updated: 2019-03-15Bibliographically approved
Maslik, J., Andersson, H., Forsberg, V., Engholm, M., Zhang, R. & Olin, H. (2018). PEDOT:PSS temperature sensor ink-jet printed on paper substrate. Paper presented at 20th International Workshop on Radiation Imaging Detectors. Journal of Instrumentation, 13, Article ID C12010.
Open this publication in new window or tab >>PEDOT:PSS temperature sensor ink-jet printed on paper substrate
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2018 (English)In: Journal of Instrumentation, ISSN 1748-0221, E-ISSN 1748-0221, Vol. 13, article id C12010Article in journal (Refereed) Published
Abstract [en]

In this work we present an ink-jet printed temperature sensor consisting of PEDOT:PSSprinted on paper suitable for packaging, flexible electronics and other printed applications. Thesubstrate showed to have a large influence on both the resistance aswell as the temperature sensitivityof the PEDOT:PSS ink. This effect is most likely due to NaCl content in the photo paper coating,which reacts with the PEDOT:PSS. The temperature coefficient of a prepared device of α = -0.030relative to room temperature (22°C) was measured, which is higher than compared to for exampleSilicon α = -0.075.

Keywords
PEDOT:PSS, printed, ink-jet, temperature sensor, paper
National Category
Other Electrical Engineering, Electronic Engineering, Information Engineering
Identifiers
urn:nbn:se:miun:diva-35247 (URN)10.1088/1748-0221/13/12/C12010 (DOI)000452801600005 ()2-s2.0-85059901876 (Scopus ID)
Conference
20th International Workshop on Radiation Imaging Detectors
Funder
Knowledge Foundation
Available from: 2018-12-17 Created: 2018-12-17 Last updated: 2019-03-15Bibliographically approved
Zhang, R., Hummelgård, M., Forsberg, V., Andersson, H., Engholm, M., Öhlund, T., . . . Olin, H. (2018). Photoconductivity of acid exfoliated and flash-light-processed MoS2 films. Scientific Reports, 8, Article ID 3296.
Open this publication in new window or tab >>Photoconductivity of acid exfoliated and flash-light-processed MoS2 films
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2018 (English)In: Scientific Reports, ISSN 2045-2322, E-ISSN 2045-2322, Vol. 8, article id 3296Article in journal (Refereed) Published
Abstract [en]

MoS2 has been studied intensively during recent years as a semiconducting material in several fields, including optoelectronics, for applications such as solar cells and phototransistors. The photoresponse mechanisms of MoS2 have been discussed but are not fully understood, especially the phenomenon in which the photocurrent slowly increases. Here, we report on a study of the photoresponse flash-light-processed MoS2 films of different thicknesses and areas. The photoresponse of such films under different light intensities and bias voltages was measured, showing significant current changes with a quick response followed by a slow one upon exposure to pulsed light. Our in-depth study suggested that the slow response was due to the photothermal effect that heats the MoS2; this hypothesis was supported by the resistivity change at different temperatures. The results obtained from MoS2 films with various thicknesses indicated that the minority-carrier diffusion length was 1.36 mu m. This study explained the mechanism of the slow response of the MoS2 film and determined the effective thickness of MoS2 for a photoresponse to occur. The method used here for fabricating MoS2 films could be used for fabricating optoelectronic devices due to its simplicity.

National Category
Physical Sciences
Identifiers
urn:nbn:se:miun:diva-33302 (URN)10.1038/s41598-018-21688-0 (DOI)000425380900079 ()29459668 (PubMedID)2-s2.0-85061713034 (Scopus ID)
Available from: 2018-03-19 Created: 2018-03-19 Last updated: 2019-03-20Bibliographically approved
Forsberg, V., Andersson, H., Engholm, M., Thungström, G., Zhang, R., Hummelgård, M., . . . Norgren, M. (2018). Photodetector of multilayer exfoliated MoS2 deposited on polyimide films. In: : . Paper presented at 20th International Workshop on Radiation Imaging Detectors, Sundsvall, 24-28 June, 2018.
Open this publication in new window or tab >>Photodetector of multilayer exfoliated MoS2 deposited on polyimide films
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2018 (English)Conference paper, Poster (with or without abstract) (Other academic)
Abstract [en]

We fabricated a photodetector based on multilayer molybdenum disulfide (MoS2) by micromechanical cleavage of a molybdenite crystal using a polyimide film. We deposited 40 nm of gold by vacuum sputtering and copper tape was used for the contacts.  Without any surface treatment, we achieved high responsivity at different incident optical power. The calculated responsivity was 23 mA/W of incident optical power in the range between 400 and 800 nm. For the responsivity measurement it was estimated that MoS2 have a bandgap of 1.6 eV, which lies between monolayer and multilayer films. The thickness of the MoS2 thin film was determined by Raman spectroscopy evaluating the difference between the in plane  and out of plane  Raman modes. The measurement of IV curves indicated Ohmic contacts in respect to the Au regardless of the incident optical power. Our device fabrication was much simpler than previous reported devices and can be used to test the light absorption and luminescence capabilities of exfoliated MoS2.

Keywords
Photodetector, MoS2
National Category
Chemical Engineering Materials Engineering Physical Sciences
Identifiers
urn:nbn:se:miun:diva-34035 (URN)
Conference
20th International Workshop on Radiation Imaging Detectors, Sundsvall, 24-28 June, 2018
Funder
Knowledge Foundation, 2600364
Available from: 2018-06-29 Created: 2018-06-29 Last updated: 2018-08-16Bibliographically approved
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Identifiers
ORCID iD: ORCID iD iconorcid.org/0000-0001-7329-3359

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